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- W2083816710 abstract "EPR measurements have been made on single crystals of CsMgCl 3 doped with iron. From x-ray irradiated samples, signals from a Fe 3+ centre with trigonal symmetry are observed. Magnitudes of the spin-Hamiltonian parameters have been determined accurately by a direct matrix-diagonalization method. Negative signs of b 0 2 and b 0 4 parameters are determined from the observation of a depopulation effect at 4.2 K. The absolute sign of the b 3 4 parameter is deduced to be negative by the use of spin-Hamiltonian separation analysis. The spectrum has been ascribed to a Fe 3+ ion substituted for a Mg 2+ ion without any charge compensators in its immediate neighbourhood. An empirical rule for the trigonally symmetric Fe 3+ centre is presented; that is, negative and positive signs of b 0 2 come respectively from trigonal elongation or compression of the ligand octahedron along the trigonal axis from the ordinary configuration. It is suggested that the magnitudes of |b 0 2 | for the Fe 3+ centre relative to those of |b 0 2 | for the corresponding Cr 3+ centre in the same matrix crystal are anomalously small in fluorides." @default.
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- W2083816710 date "2005-02-12" @default.
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- W2083816710 title "An electron paramagnetic resonance study of a trigonally symmetric Fe3+centre in CsMgCl3single crystal" @default.
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- W2083816710 doi "https://doi.org/10.1088/0953-8984/17/8/016" @default.
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