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- W2083928633 abstract "The activity coefficient of oxygen $$ f_{text{O}}^{0} $$ in liquid Ag and binary Ag–Te dilute alloys were determined between 1,285 and 1,485 K by coulometric titration using the electrochemical cell (Ir, [O] in liquid metal or alloy | yttria stabilized zirconia | air, Pt). The experimental and evaluation procedures described in the literature were adopted. The oxygen activity coefficient was determined in pure liquid silver to be $$ln f_{text{O}}^0 = {{ - 1{,}760.2} mathord{left/ {vphantom {{ - 1,760.2} T}} right. kern-nulldelimiterspace} T} + 0.6315$$ . Next, the oxygen activity coefficient in dilute Ag–(Te)–O alloys for variable X Te content (from 0.01 to 0.06) was measured. From the obtained results, Wagner’s interaction parameter $$ varepsilon_{text{O}}^{text{Te}} $$ as a function of temperature was derived in the form $$varepsilon _{text{O}}^{{text{Te}}} left( { pm 0.32} right) = {{ - 18,483} mathord{left/ {vphantom {{ - 18,483} T}} right. kern-nulldelimiterspace} T} + 7.668$$ . The electrochemical coulometric titration method seems to be very useful to study the thermodynamics of oxygen interaction in liquid silver and its alloys." @default.
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- W2083928633 date "2012-08-25" @default.
- W2083928633 modified "2023-10-14" @default.
- W2083928633 title "Thermodynamics of oxygen in dilute liquid silver–tellurium alloys" @default.
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- W2083928633 doi "https://doi.org/10.1007/s00706-012-0771-z" @default.
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