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- W2084058544 abstract "The two-dimensional version of a mesoscale meteorological model is applied to the removal of soluble and reactive species by orographically forced clouds and precipitation. The model includes both SO42- and acidity productions within typical maritime clouds. A quasi-spectral microphysical scheme allows for a detailed description of the partitioning of different constituents between air, cloud and rain. Model results indicate that this partitioning is influenced by the solubility and the reactivity of the species, and also by microphysical processes. The sharing of dissoved species between cloud and rain is found to be different upwind and downwind from the mountain top, leading to higher acidity in rain downstream. Replenishment of new material into the cloud through advection, aerosol load through nucleation, chemical factors and microphysical processes all compete to affect the resultant acidity in cloud-water and rain-water. Model estimates for these overlying processes suggest that interaction between dynamics, microphysics and chemistry must be well represented to predict cloud and rain compositions." @default.
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- W2084058544 date "1990-01-01" @default.
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- W2084058544 title "Mesoscale modeling of acidity production in orographic clouds and rain" @default.
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- W2084058544 doi "https://doi.org/10.1016/0960-1686(90)90065-u" @default.
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