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• W2084452908 abstract "We demonstrate an enhancement of photocurrent in hybrid photovoltaic cells based on nanoparticles of zinc oxide (ZnO) and poly(3-hexylthiophene) (P3HT), through molecular interface modification with and without cis-bis(4,4′-dicarboxy-2,2′bipyridine) ruthenium (II) (N3-dye) and α-Sexithiophen-2-yl-phosphonic Acid (6TP) as interface modifiers. We identify the formation of long-lived polarons at P3HT:ZnO interface by means of quasi-steady-state photoinduced absorption (PIA) spectroscopy. Furthermore, by probing the pump-modulation-frequency-dependent PIA signal, we find that P3HT:ZnO-N3 and P3HT:ZnO-6TP exhibit more sharply decaying density with increasing modulation frequency, which is indicative of a longer average lifetime, approximating 1 ms as opposed to ∼0.2 ms without ZnO surface modification. This highlights the importance of the molecular interface modification in the steady-state polaron dynamics in hybrid solar cells." @default.
• W2084452908 created "2016-06-24" @default.
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• W2084452908 date "2014-08-19" @default.
• W2084452908 modified "2023-10-17" @default.
• W2084452908 title "The influence of molecular interface modification on the charge dynamics of polymeric semiconductor:ZnO heterostructure" @default.
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• W2084452908 doi "https://doi.org/10.1063/1.4893361" @default.
• W2084452908 hasPublicationYear "2014" @default.
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