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- W2084497613 abstract "High optical quality samples of polydimethylsiloxane rubber have been prepared, crosslinked by γ radiation. The raman depolarization rations,ϱ, of two highly polarized bands, the CH 3 stretching at 2907 cm −1 and the Si — O skeletal mode at 491 cm −1 , have been measured as a function of temperature and strain. The changes in ϱ are related to changes in the relative populations of trans and gauche isomer population, and a value for Δ E , the energy difference, is found to be 820 +50 −20 cal/mole. The proportionality constant in a theory connecting strain and isomer populations D 2 is measured to be 10 ± 2. Computer calculations based on statistical weight matrices yield Δ E = 875 cal/mole and D 2 = 1.18. Reasons for the discrepancy in the D 2 values are discussed." @default.
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- W2084497613 date "1973-12-01" @default.
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- W2084497613 title "Investigation of molecular isomerism in polydimethylsiloxane by raman scattering" @default.
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- W2084497613 doi "https://doi.org/10.1016/0301-0104(73)80018-7" @default.
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