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- W2084611482 abstract "High-temperature experiments were performed behind reflected shock waves using SiH4, SiH4/O2, H2/O2, SiH4/H2/O2, CH4/O2, and SiH4/CH4/O2 mixtures highly diluted in argon. Reflected-shock temperatures ranged from 1050—2250 K at a pressure near 1 atm. Reaction progress was monitored by observing the time histories of several species, including OH*, SiH4, SiH2, and CH* using emission and laser absorption techniques. The oxidation and ignition data are reported in the form of species concentration profiles and plots of characteristic times as a function of temperature. The species time histories exhibit a dual oxidation behavior for most of the fuel/O2/SiH4 experiments, indicating the silane reacts first followed by reaction of the fuel with the remaining oxygen. As expected, the presence of silane in the fuel/O2 mixtures markedly reduced the ignition delay time, usually by a factor of two or more even at molar SiH4 concentrations as low as 1% of the fuel concentration. The database presented herein can be used to validate chemical kinetics models of hightemperature silane oxidation for propulsion and materials processing applications." @default.
- W2084611482 created "2016-06-24" @default.
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- W2084611482 date "2002-07-07" @default.
- W2084611482 modified "2023-09-25" @default.
- W2084611482 title "Ignition and Oxidation of Dilute Silane-Oxidizer Mixtures Behind Reflected Shock Waves" @default.
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- W2084611482 doi "https://doi.org/10.2514/6.2002-3875" @default.
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