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• W2084669405 startingPage "1683" @default.
• W2084669405 abstract "Abstract Using a group of six neutral M II Cl 2 ‐containing coordination compounds as building blocks, the first systematic investigation of CH⋅⋅⋅Cl hydrogen‐bonding interactions was performed. Single‐crystal X‐ray structural analyses of four new compounds (pseudo‐tetrahedral Co II and Zn II ; distorted trigonal bipyramidal Zn II ) authenticate the metal coordination geometry. To provide a unified view of the presence of noncovalent interactions in this class of compounds, we have re‐examined the packing diagram of two previously reported compounds (a distorted square‐pyramidal Cu II complex and a trans ‐octahedral Co II complex). The organic ligands of our choice comprise bidentate/tridentate pyrazolylmethylpyridines and an unsymmetrical tridentate pyridylalkylamine. This systematic investigation has allowed us to demonstrate the existence of versatile CH⋅⋅⋅Cl 2 M interactions and to report the successful application of such units as inorganic supramolecular synthons. Additional noncovalent interactions such as CH⋅⋅⋅O and OH⋅⋅⋅Cl hydrogen bonding and π–π stacking interactions have also been identified. Formation of novel supramolecular architectures has been revealed: 2D lamellar ( p ‐cyclophane) and 3D lamellar, 3D “stitched staircase” (due to additional hydrogen‐bonding interactions by water tetramers, with an average OO bond length in the tetramer unit of 2.926 Å, acting as “molecular clips” between staircases), 3D linked ladder, and single‐stranded 1D helix." @default.
• W2084669405 created "2016-06-24" @default.
• W2084669405 creator A5015342021 @default.
• W2084669405 creator A5043033059 @default.
• W2084669405 creator A5058011193 @default.
• W2084669405 date "2004-03-24" @default.
• W2084669405 modified "2023-10-18" @default.
• W2084669405 title "First Systematic Investigation of CH⋅⋅⋅Cl Hydrogen Bonding Using Inorganic Supramolecular Synthons: Lamellar, Stitched Stair-Case, Linked-Ladder, and Helical Structures" @default.
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• W2084669405 doi "https://doi.org/10.1002/chem.200305701" @default.
• W2084669405 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15054755" @default.
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