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• W2084996987 abstract "The rotational predissociation of water molecules in the vibrationless level of the B1 state was investigated under jet-cooled conditions (27—154 K) by exciting them with a tunable VUV laser in the wavelength range of 124.3—123.7 nm and by detecting the total fluorescence from electronically excited photofragments OH(A2Σ+). Due to the simple one-photon selection rule and the efficient rotational cooling, individual low-J rotational transitions of the B1–A1 origin band were observed with almost no overlap in the laser-induced photofragment fluorescence (LIPF) spectrum. The widths and intensities of these rotational transitions exhibited pronounced dependence on the parent rotational levels in the B1 state. The least-squares analysis of the observed line-widths (FWHM) of the resolved rotational transitions, Γ ’s, showed that they are well described by the formula, Γ = Γ0 + αa , with optimized parameters Γ0 = 2.5(1) cm−1 and αa = 0.63(1) cm−1, indicating that (i) the homogeneous interaction couples the ..." @default.
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• W2084996987 date "1998-02-01" @default.
• W2084996987 modified "2023-09-25" @default.
• W2084996987 title "Rotational Predissociation Dynamics of H₂O (C¹B₁) by VUV Laser-Induced Photofragment Fluorescence Spectroscopy" @default.
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• W2084996987 doi "https://doi.org/10.1246/bcsj.71.355" @default.
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