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- W2085102092 abstract "Abstract The equilibrium constant for the reaction, ThF4(s) + SiO2(s) ⇌ ThO2(s) + SiF4(g) was determined over the temperature interval 871°–1077°K by measuring the equilibrium pressure of SiF4 above the system. The pressure of SiF4 from this reaction is given by log P (atm) = −8200 ± 120 T(∘K) + 7.740 ± 0.130. A heat capacity correction of −2·76 cal deg−1 mole−1 gives for the reaction at 298°K, ΔF° = 27·9 kcal/mole, ΔH° = 39·4 kcal/mole, and ΔS° = 38·7 cal deg−1mole−1. From these and existing thermodynamic data for SiO2, ThO2 and SiF4 the ΔF°, ΔH° and ΔS° of formation of ThF4 from the elements at 298°K were calculated to be −459·9 kcal/mole, −482·4 kcal/mole and −75·8 cal deg−1 mole−1, respectively." @default.
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- W2085102092 date "1960-10-01" @default.
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- W2085102092 title "The free energy, heat and entropy of formation of thorium tetrafluoride" @default.
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