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- W2085105965 abstract "Abstract We present direct evidence for the formation of nitrites/HONO in the oxidative activation of NO over Fe-zeolites. Exposure of a Fe-ZSM-5 + BaO/Al 2 O 3 physical mixture to NO + O 2 at 120 °C resulted in forming nitrites on Fe-sites and trapping them on BaO via gas-phase equilibrium with HONO. Identification of nitrites was confirmed by: (i) their thermal decomposition to an equimolar mix of NO and NO 2 during TPD, (ii) N 2 formation during their reaction with NH 3 at 120 °C, (iii) ex situ IR analysis of the BaO powder after discharge and separation of the mechanical mixture. The reactivity data suggest that nitrites/HONO are intermediates both in the NO oxidation to NO 2 and in the Standard SCR reactions." @default.
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- W2085105965 date "2014-03-01" @default.
- W2085105965 modified "2023-09-26" @default.
- W2085105965 title "Identification of nitrites/HONO as primary products of NO oxidation over Fe-ZSM-5 and their role in the Standard SCR mechanism: A chemical trapping study" @default.
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- W2085105965 doi "https://doi.org/10.1016/j.jcat.2013.11.028" @default.
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