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- W2085190438 abstract "A method to derive experimentally the configurational entropy that governs the structural relaxation process in supercooled (supercompressed) liquids is presented. Light scattering, dielectric, calorimetric and dilatometric measure-ments are used to test the method in o-terphenyl. The combined analysis of relaxation data as a function of temperature and pressure is found to be essential to quantify a realistic value of the non-structural thermal expansion and the configurational entropy of the system. The latter is estimated as a fraction of the excess entropy of the liquid over its stable crystalline phase. Our results indicate that the number of configurations connected to the structural relaxation contributes approximately 70% to the excess entropy." @default.
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- W2085190438 date "2004-05-01" @default.
- W2085190438 modified "2023-09-26" @default.
- W2085190438 title "Configurational and excess entropies in a fragile glass former and their relation with structural relaxation" @default.
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- W2085190438 doi "https://doi.org/10.1080/14786430310001644291" @default.
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