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- W2085283048 abstract "The formation of NH 2, ads and its further reactions with hydrogen and NO on the Pt(100) surface were previously studied by the methods of HREELS and TPR, in order to understand the role of amino species in the mechanism of the NO + H 2 reaction. In this work the method of unity bond index – quadratic exponential potential (UBI-QEP) has been employed to rationalize the experimental findings by calculating the energies associated with the envisaged routes of reactions. It is concluded that the activation energy of formation of NH 2, ads is higher than water production. The simplicity of recombinative desorption of N 2 is due to the decrease of its activation energy because of the destabilizing effect of O ads and NO ads . The rate-determining step of explosive surface reaction in the saturated coadsorption layer of NH 2, ads and NO ads is dissociation of NO ads . Autocatalytic acceleration of the explosive reactions is due to the decrease of activation energy of the rds by increasing the number adsorption vacant sites. H 2 O is produced via two different processes with different activation energies. NH 3 is produced via several paths." @default.
- W2085283048 created "2016-06-24" @default.
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- W2085283048 date "2003-08-01" @default.
- W2085283048 modified "2023-09-26" @default.
- W2085283048 title "Investigation of the Energetics of the Reactions of NH2 Species with Hydrogen and NO on the Pt(100) Surface by the Method of UBI-QEP" @default.
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- W2085283048 doi "https://doi.org/10.1142/s0218625x03005347" @default.
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