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- W2085304037 abstract "5-Hydroxymethyl furfural is an important platform chemical. It is successfully synthesized from renewable carbohydrates using mesoporous AlSBA-15 catalysts under biphasic conditions. Fine tuning of the catalyst acidity is important to drive the reaction to give good yields of furan compound. Al-SBA-15 catalysts with different Si/Al ratios were prepared and characterized by XRD, 27Al MASNMR, SEM, TEM, N2 sorption, ICP-OES and TPD of ammonia. Results show that part of aluminium is substituted into tetrahedral positions. The catalyst with lower acid site density but medium to strong acidstrength favours selective formation of HMF. Under the optimized conditions, HMF selectivity was as high as 88% at 59 mol% conversion of fructose. Leaching of part of aluminium occurs under hydrothermal conditions, if solvent mixtures containing water are used, while activity can be retained if DMSO is used as solvent." @default.
- W2085304037 created "2016-06-24" @default.
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- W2085304037 date "2013-11-01" @default.
- W2085304037 modified "2023-10-07" @default.
- W2085304037 title "Dehydration of fructose to 5-hydroxymethyl furfural over ordered AlSBA-15 catalysts" @default.
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- W2085304037 doi "https://doi.org/10.1016/j.micromeso.2013.07.015" @default.
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