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- W2085375784 abstract "This paper reports a reduced mechanism used in urea-based SNCR process for NOx control that is developed from the detailed mechanism originally proposed by Rota et al. (Chem. Eng. Sci. 2002, 57, 27−38) consisting of 173 elemental reactions and 31 chemical species. Sensitivity analysis and rate-of-production analysis are first conducted to exclude redundant elemental reactions and species, forming a skeletal mechanism. After that, quasi-steady-state species are identified and a 12-step 16-species reduced mechanism is established. The balance equations for quasi-steady-state species are innovatively solved by means of QSS graph method presented by Lu and Law (J. Phys. Chem. A 2006, 110, 13202−13208) with the avoidance of efficiency compromise stemming from algebraic iterations. The predictions of the reduced mechanism show satisfactory agreement with those of the detailed one over a wide range of operating conditions, including various temperatures, molar ratio of CO(NH2)2/NO and O2 and CO concentrations. The performances of QSS graph method and traditional QSSA by iteration are compared in plug-flow computations. The deviation in accuracy is only in order of 0.01%, while QSS graph creates nearly 40% speed-up significantly superior to QSSA by iteration." @default.
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- W2085375784 date "2009-07-16" @default.
- W2085375784 modified "2023-09-26" @default.
- W2085375784 title "Development and Validation of a Reduced Mechanism for Urea-based SNCR Process based on QSS Graph" @default.
- W2085375784 doi "https://doi.org/10.1021/ef900165k" @default.
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