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- W2085502314 abstract "Gold nanoparticles have been adsorbed as monolayers on silicon and glass substrates and the structure evolution following femtosecond laser excitation has been analyzed by means of time resolved X-ray scattering. The synchronization of the laser to the X-ray pulse structure emitted from a third generation synchrotron source allows to obtain a natural time resolution of 100 ps for the lattice kinetics. The prospects of using a picosecond X-ray streak camera are explored. The lattice kinetics are dominated by the fast heating of the particle lattice and nanosecond cooling times. However, the analysis of peak shapes reveals the presence of nonthermal motion within the lattice. Unexpectedly large relaxation times for the thermalization of vibrational modes are found and are attributed to the weak mechanical coupling to the substrate. Strong nonuniform strain develops within the domain of electron–phonon interaction time regime after the laser excitation as seen with the X-ray streak camera." @default.
- W2085502314 created "2016-06-24" @default.
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- W2085502314 date "2004-04-01" @default.
- W2085502314 modified "2023-09-26" @default.
- W2085502314 title "Structural kinetics of laser-excited metal nanoparticles supported on a surface" @default.
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- W2085502314 doi "https://doi.org/10.1016/j.chemphys.2003.10.041" @default.
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