Matches in SemOpenAlex for { <https://semopenalex.org/work/W2085511957> ?p ?o ?g. }
- W2085511957 endingPage "3684" @default.
- W2085511957 startingPage "3684" @default.
- W2085511957 abstract "We designed and synthesized a perfluorinated covalent triazine-based framework (FCTF-1) for selective CO2 capture. The incorporation of fluorine (F) groups played multiple roles in improving the framework's CO2 adsorption and separation capabilities. Thermodynamically, the strongly polar C–F bonds promoted CO2 adsorption via electrostatic interactions, especially at low pressures. FCTF-1's CO2 uptake was 1.76 mmol g−1 at 273 K and 0.1 bar through equilibrium adsorption, exceeding the CO2 adsorption capacity of any reported porous organic polymers to date. In addition, incorporating F groups produced a significant amount of ultra-micropores (<0.5 nm), which offered not only high gas adsorption potential but also kinetic selectivity for CO2–N2 separation. In mixed-gas breakthrough experiments, FCTF-1 exhibited an exceptional CO2–N2 selectivity of 77 under kinetic flow conditions, much higher than the selectivity (31) predicted from single-gas equilibrium adsorption data. Moreover, FCTF-1 proved to be tolerant to water and its CO2 capture performance remained excellent when there was moisture in the gas mixture, due to the hydrophobic nature of the C–F bonds. In addition, the moderate adsorbate–adsorbent interaction allowed it to be fully regenerated by pressure swing adsorption processes. These attributes make FCTF-1 a promising sorbent for CO2 capture from flue gas." @default.
- W2085511957 created "2016-06-24" @default.
- W2085511957 creator A5018172419 @default.
- W2085511957 creator A5023896611 @default.
- W2085511957 creator A5037709424 @default.
- W2085511957 creator A5043238555 @default.
- W2085511957 creator A5091448543 @default.
- W2085511957 date "2013-01-01" @default.
- W2085511957 modified "2023-10-06" @default.
- W2085511957 title "A perfluorinated covalent triazine-based framework for highly selective and water–tolerant CO2 capture" @default.
- W2085511957 cites W1909940713 @default.
- W2085511957 cites W1966865995 @default.
- W2085511957 cites W1968876938 @default.
- W2085511957 cites W1971819215 @default.
- W2085511957 cites W1974314684 @default.
- W2085511957 cites W1975507538 @default.
- W2085511957 cites W1975618709 @default.
- W2085511957 cites W1975694604 @default.
- W2085511957 cites W1976416233 @default.
- W2085511957 cites W1976711248 @default.
- W2085511957 cites W1979703303 @default.
- W2085511957 cites W1982860645 @default.
- W2085511957 cites W1982981013 @default.
- W2085511957 cites W1986575958 @default.
- W2085511957 cites W1987581091 @default.
- W2085511957 cites W1989524946 @default.
- W2085511957 cites W1995543239 @default.
- W2085511957 cites W1997402316 @default.
- W2085511957 cites W2002405030 @default.
- W2085511957 cites W2002905537 @default.
- W2085511957 cites W2005005410 @default.
- W2085511957 cites W2006215520 @default.
- W2085511957 cites W2011579724 @default.
- W2085511957 cites W2019832034 @default.
- W2085511957 cites W2021208541 @default.
- W2085511957 cites W2021681230 @default.
- W2085511957 cites W2024506042 @default.
- W2085511957 cites W2028182782 @default.
- W2085511957 cites W2028323767 @default.
- W2085511957 cites W2029366295 @default.
- W2085511957 cites W2031776732 @default.
- W2085511957 cites W2044062160 @default.
- W2085511957 cites W2047433606 @default.
- W2085511957 cites W2047483519 @default.
- W2085511957 cites W2047640646 @default.
- W2085511957 cites W2048575095 @default.
- W2085511957 cites W2049145344 @default.
- W2085511957 cites W2049524352 @default.
- W2085511957 cites W2050821402 @default.
- W2085511957 cites W2052703700 @default.
- W2085511957 cites W2052886839 @default.
- W2085511957 cites W2053118165 @default.
- W2085511957 cites W2054886106 @default.
- W2085511957 cites W2055738871 @default.
- W2085511957 cites W2058930892 @default.
- W2085511957 cites W2060676355 @default.
- W2085511957 cites W2062904068 @default.
- W2085511957 cites W2063106084 @default.
- W2085511957 cites W2066214067 @default.
- W2085511957 cites W2067658025 @default.
- W2085511957 cites W2070821099 @default.
- W2085511957 cites W2074200154 @default.
- W2085511957 cites W2074211433 @default.
- W2085511957 cites W2079588474 @default.
- W2085511957 cites W2092153004 @default.
- W2085511957 cites W2092538171 @default.
- W2085511957 cites W2094005838 @default.
- W2085511957 cites W2094145140 @default.
- W2085511957 cites W2094286279 @default.
- W2085511957 cites W2104015519 @default.
- W2085511957 cites W2108510319 @default.
- W2085511957 cites W2114423620 @default.
- W2085511957 cites W2125053394 @default.
- W2085511957 cites W2126430743 @default.
- W2085511957 cites W2128705258 @default.
- W2085511957 cites W2130849112 @default.
- W2085511957 cites W2131503876 @default.
- W2085511957 cites W2148295263 @default.
- W2085511957 cites W2150021001 @default.
- W2085511957 cites W2151588032 @default.
- W2085511957 cites W2152291440 @default.
- W2085511957 cites W2158415514 @default.
- W2085511957 cites W2160618941 @default.
- W2085511957 cites W2166093634 @default.
- W2085511957 cites W2167154209 @default.
- W2085511957 cites W2168175046 @default.
- W2085511957 cites W2168614264 @default.
- W2085511957 cites W2172052812 @default.
- W2085511957 cites W2313030436 @default.
- W2085511957 cites W2313379369 @default.
- W2085511957 cites W2313549007 @default.
- W2085511957 cites W2316488167 @default.
- W2085511957 cites W2318712254 @default.
- W2085511957 cites W2325161613 @default.
- W2085511957 cites W2325538496 @default.
- W2085511957 cites W2326172743 @default.
- W2085511957 cites W2327837350 @default.
- W2085511957 cites W2331279123 @default.