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- W2085709711 abstract "Ordered mesoporous zinc-doped SnO2 (Zn-doped meso-SnO2) particles with a high surface area and a 2D hexagonal-type pore structure are synthesized by a double-replication procedure using SBA-15 silica and CMK-3 carbon as successive hard templates. The double-replication procedure provides large mesopores (diameter ∼10 nm), which are essential in dye-sensitized solar cells (DSCs) for the facile diffusion of redox electrolytes. It is shown that Zn doping into an ordered mesoporous SnO2 framework induces a negative shift in the flat-band potential (VFB) and also increases the isoelectric point. Consequently, DSCs employing Zn-doped meso-SnO2 photoanodes demonstrate longer electron lifetimes and increased dye loading than their undoped meso-SnO2 counterparts. A maximum energy-conversion efficiency (η) of 3.73% is achieved from solar cells fabricated with 3 mol% Zn-doped meso-SnO2 photoanodes, a nearly five-fold improvement compared to undoped meso-SnO2 photoanode DSCs (η = 0.81%)." @default.
- W2085709711 created "2016-06-24" @default.
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- W2085709711 date "2011-01-01" @default.
- W2085709711 modified "2023-09-25" @default.
- W2085709711 title "Ordered mesoporous Zn-doped SnO2 synthesized by exotemplating for efficient dye-sensitized solar cells" @default.
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- W2085709711 doi "https://doi.org/10.1039/c1ee01123e" @default.
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