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- W2085711704 abstract "Electron-trapped ${mathrm{Fe}}^{+}$-type centers, produced by x-ray irradiation at $80phantom{rule{0.3em}{0ex}}mathrm{K}$ and further annealing at higher temperatures in iron-doped ${mathrm{SrCl}}_{2}$ single crystals grown in chlorine gas, have been investigated by electron paramagnetic resonance. The ${mathrm{Fe}}^{+}(mathrm{III})$ and ${mathrm{Fe}}^{+}(mathrm{IIIa})$ centers, produced by annealing at temperatures higher than $200phantom{rule{0.3em}{0ex}}mathrm{K}$, exhibit monoclinic local symmetry with the two $stackrel{⃡}{g}$- tensor principal axes situated in the (110) plane slightly tilted away from the [001] and [1--10] directions, respectively. The ${mathrm{Fe}}^{+}(mathrm{IV})$ center, observed after several cycles of irradiation and annealing to $700phantom{rule{0.3em}{0ex}}mathrm{K}$, exhibits tetragonal local symmetry around $⟨100⟩$ and a well-resolved four-component structure, attributed to the superhyperfine interaction with a neighboring monovalent impurity ion. The presence and properties of the low symmetry radiation-induced ${mathrm{Fe}}^{+}$ paramagnetic centers are attributed to trapping and the thermally activated movement of chlorine interstitials. Both precursor ${mathrm{Fe}}^{2+}$ and resulting ${mathrm{Fe}}^{+}$ centers are perturbed by these interstitials, which are introduced in ${mathrm{SrCl}}_{2}:mathrm{Fe}$ crystals during growth under a chlorine atmosphere." @default.
- W2085711704 created "2016-06-24" @default.
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- W2085711704 date "2006-05-01" @default.
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- W2085711704 title "Electron-trapping centers and interstitials in chlorinatedSrCl2:Fesingle crystals" @default.
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- W2085711704 doi "https://doi.org/10.1103/physrevb.73.174103" @default.
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