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- W2085752883 abstract "Within the framework of a generalized operator transform technique the problem of the calculation of (time-proportional) transition probabilities of ESR, ENDOR and electron—nuclear multiple-resonance (ENmMR) transitions to first-order Rayleigh—Schrödinger perturbation theory is treated. Fermi's golden rule is extended to spin systems subject (besides the microwave field) to several (weak) coherent or non-coherent radio-frequency fields (monochromatic or narrowband modulated). It is shown that for recently introduced experimental techniques using either circularly polarized or polarization-modulated radio-frequency fields (CP ENDOR and PM ENDOR, respectively), both modulus and phase of the transition matrix elements for each radio-frequency field are required. Based on the first-order basis functions, analytical expressions for ESR and ENDOR transition probabilities for a general spin hamiltonian and various modulation schemes are given, which explicitly contain both zeroth- and first-order (“hyperfine enhancement”) contributions. The accuracy of the analytical first-order expressions is tested for two spin systems and found to be in excellent agreement with exact numerical calculations." @default.
- W2085752883 created "2016-06-24" @default.
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- W2085752883 date "1982-08-01" @default.
- W2085752883 modified "2023-10-03" @default.
- W2085752883 title "Transition probabilities in electron—nuclear double- and multiple-resonance spectroscopy with non-coherent and coherent radio-frequency fields" @default.
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- W2085752883 doi "https://doi.org/10.1016/0301-0104(82)85099-4" @default.
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