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• W2085780566 abstract "A thermodynamic model has been developed which predicts the growth of either an initial (semi)coherent, strained crystalline oxide phase, or an initial amorphous oxide phase (with a possible amorphous-to-crystalline transition) on the bare single-crystalline metal substrate as a function of the metal substrate orientation, the growth temperature, and the oxide-film thickness. The model accounts for relaxation of residual stresses in a crystalline oxide overgrowth by plastic deformation (i.e., through the introduction of misfit dislocations at the metal/oxide interface). As an example, the microstructural evolution of the initial oxide film grown on the {111}, {110}, and {100} crystallographic surfaces of a bare Cr substrate has been modeled as a function of the growth temperature and the oxide-film thickness $(<5phantom{rule{0.3em}{0ex}}mathrm{nm})$. The initial oxide-film growth on the bare Cr{100} and Cr{111} substrates is predicted to proceed by the initial formation and growth of an amorphous oxide film up to a critical thickness of about 0.5 and $0.9phantom{rule{0.3em}{0ex}}mathrm{nm}$, respectively. On the other hand, the onset of oxidation on a bare Cr{110} substrate should proceed by the direct overgrowth of a semicoherent, strained crystalline oxide film. These model predictions provide understanding for experimental observations reported in the literature." @default.
• W2085780566 created "2016-06-24" @default.
• W2085780566 creator A5028856141 @default.
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• W2085780566 date "2006-10-17" @default.
• W2085780566 modified "2023-09-27" @default.
• W2085780566 title "Thermodynamic model of oxide overgrowth on bare metals: Relaxation of growth strain by plastic deformation" @default.
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• W2085780566 doi "https://doi.org/10.1103/physrevb.74.144103" @default.
• W2085780566 hasPublicationYear "2006" @default.
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