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- W2085959477 abstract "A critical examination is made of the Birge-Sponer method of determining dissociation energies of diatomic molecules. Dissociation energies of certain classes of molecules as determined by linear extrapolation are compared with values determined independently. For the ground states of ordinary molecules the linear extrapolation tends to give too high results, often by around 20%. For molecules in which ionic binding is important the extrapolation often comes too low, sometimes much too low. For the molecules in which one atom has a 1S0 ground state the linear extrapolation is much too high. The method appears to work satisfactorily for ionized molecules. Excited states of molecules cannot, in general, be relied on to give good extrapolations. These empirical observations are discussed in terms of the potential-energy curves and the binding forces in the molecules at large inter-nuclear distances." @default.
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- W2085959477 date "1946-09-01" @default.
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- W2085959477 title "The determination of dissociation energies by the birge-sponer extrapolation" @default.
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- W2085959477 doi "https://doi.org/10.1088/0959-5309/58/5/302" @default.
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