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• W2086081572 abstract "The species HNCS and NCS have been studied by photoionization mass spectroscopy. The adiabatic ionization potential (IP) of HNCS is ≤9.92 eV; the shape of the ion yield curve near threshold implies a large change in geometry, perhaps to linear HNCS+. Various appearance potentials (AP) from HNCS are determined by a more objective procedure, from which ΔH○f(HNCS)≳29.6 kcal/mol (and very likely ≥31.0±0.7 kcal/mol) is deduced. The adiabatic IP of NCS is 10.689±0.005 eV. This quantity, together with AP(NCS+/HNCS), yields D0(H–NCS)≤97.2±0.2 kcal/mol. However, a measurement of the appearance potential of NCS+ from (NCS)2 results in a still lower value, D0(H–NCS)≤93.3±1.1 kcal/mol, and ΔHf0○(NCS) ≤ 72.7 ± 0.8 kcal/mol. Approximate values are obtained for ΔHf0○(HNCS+) and for the proton affinity of NCS." @default.
• W2086081572 created "2016-06-24" @default.
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• W2086081572 date "1994-11-01" @default.
• W2086081572 modified "2023-10-11" @default.
• W2086081572 title "The H–NCS bond energy, Δ<i>H</i>○<i>f</i> (HNCS), Δ<i>H</i>○<i>f</i> (NCS), and IP(NCS) from photoionization mass spectrometric studies of HNCS, NCS, and (NCS)2" @default.
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• W2086081572 doi "https://doi.org/10.1063/1.468495" @default.
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