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- W2086377665 abstract "The influence of the ac Stark effect on the line shift and line shape is studied in the three-photon resonance enhanced ionization spectroscopy of COA 1Π(v′)←X 1Σ(v″=0), where v′=1, 2, or 3. Experimental results show that the line shift varies from one vibrational band to another and differs for various lines in the same band, although it is to a lesser degree. This is given an adequate theoretical elucidation. A detailed calculation, based on the ac stark effect with evaluation of the dipole matrix element, gives −0.66, −0.31, and 0.87 cm−1 for P11 of the (1−0), (2−0), and (3−0) band, respectively, where the negative values stand for red shift while the positive one for blue shift. These results are very close to the experimental observations, viz., −0.48, −0.13, and 0.77 for P11 of the (1−0), (2−0), and (3−0) bands, respectively. Furthermore, the line shape is found to be asymmetrically broadened. For the blue-shift line, the red side is much steeper than the blue side, whereas for the red-shift line, the reverse situation appears. This is again explained as due to the ac Stark effect coupled with the spatial inhomogeneity of the laser field. According to this model, a numerical calculation for the line shape is provided which gives fairly good agreement with the experimental observation." @default.
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- W2086377665 date "1994-02-01" @default.
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- W2086377665 title "Three-photon resonance-enhanced ionization spectroscopy of CO(<i>A</i> 1Π←<i>X</i> 1Σ+). II. Line shift/profile and the ac Stark effect" @default.
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