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- W2086388745 abstract "Carbon monoxide adsorption at 80 K on γ-Al2O3, α-Cr2O3, TiO2 (rutile), SiO2-Al2O3, MgO and CeO2 was studied by transmission IR spectroscopy. It is shown that individual frequency shifts for the various types of surface OH groups when they are engaged in H-bonding interaction with CO, can be resolved. Heats of adsorption can be estimated from these shifts and a relative acidity scale for the different OH groups on a given oxide can thus be established. It is demonstrated that the high-frequency OH groups on γ-Al2O3 and α-Cr2O3 do not interact with CO, while the low-frequency groups do form H-bonds. The surface OH groups on MgO and CeO2 are too basic and remain unperturbed by CO. SiO2-Al2O3 behaved similar to SiO2 and all OH groups on rutile appear to possess sufficient proton donor strength for H-bond formation with CO." @default.
- W2086388745 created "2016-06-24" @default.
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- W2086388745 date "1987-04-01" @default.
- W2086388745 modified "2023-10-16" @default.
- W2086388745 title "Carbon monoxide — A low temperature infrared probe for the characterization of hydroxyl group properties on metal oxide surfaces" @default.
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- W2086388745 doi "https://doi.org/10.1016/0254-0584(87)90056-3" @default.
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