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- W2086882008 abstract "A model has been developed to give reliable long-term predictions for the rate of material loss from radioactive waste solids and glasses exposed to aqueous environments. The model takes into full account the effects of the interaction of the glass with the medium over the entire range of flow/dilution conditions expected in geological repositories. These effects include an increase in leach rate with decreasing rate of flow at the moderate flow region due to a pH excursion, and a subsequent decrease in leach rate at the low flow rate region due to growing saturation with respect to SiO2 Al2O3, etc. The surface-to-volume ratio can be treated as a scaling factor. The model makes possible a direct calculation of the fractional annual loss which the waste form undergoes over the entire range of possible respository conditions. The necessary data-base is obtained from the steady-state leachate concentrations measured in short-term flow tests carried out at several easily attainable combinations of experimental S/ V ratios and flow rates." @default.
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- W2086882008 date "1982-01-01" @default.
- W2086882008 modified "2023-10-17" @default.
- W2086882008 title "A flow model for the kinetics of dissolution of nuclear waste glasses" @default.
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- W2086882008 doi "https://doi.org/10.1016/0191-815x(82)90023-7" @default.
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