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- W2086953431 abstract "Electrochemical ammonia synthesis from steam and nitrogen has been systematically investigated using a proton-conducting electrolyte supported cell based on 20 mol% yttrium doped barium zirconate (BaZr0.8Y0.2O3−δ) in a temperature range of 475–600 °C at atmospheric pressure. Silver (Ag), platinum (Pt), and lanthanum strontium cobalt ferrite (La0.6Sr0.4Co0.2Fe0.8O3−δ) are used for both anode and cathode electrocatalysts. Maximum ammonia formation rates of 4.9 × 10−11 mol cm−2 s−1 and 8.5 × 10−11 mol cm−2 s−1 are observed for Ag and La0.6Sr0.4Co0.2Fe0.8O3−δ electrocatalysts, respectively, when a voltage of 0.8 V is applied. However, Pt electrocatalyst shows a negligible ammonia formation rate lower than 1 × 10−12 mol cm−2 s−1. This is ascribed to the high activity of Pt for the hydrogen evolution reaction rather than the ammonia formation reaction. The conversion efficiency of all electrocatalysts is below 1%, primarily due to the limited nitrogen disassociation activity of the electrocatalysts." @default.
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- W2086953431 date "2015-06-01" @default.
- W2086953431 modified "2023-10-18" @default.
- W2086953431 title "Electrochemical ammonia synthesis from steam and nitrogen using proton conducting yttrium doped barium zirconate electrolyte with silver, platinum, and lanthanum strontium cobalt ferrite electrocatalyst" @default.
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- W2086953431 doi "https://doi.org/10.1016/j.jpowsour.2015.03.002" @default.
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