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- W2087195685 abstract "Dissociative adsorption of hydrogen on a Fe(110) surface below 300 K. causes the formation of ordered overlayer structures as monitored by a fast Video LEED system enabling minimization of electron beam and contamination effects. Up to a hydrogen coverage of θ = 0.5 a c(2 × 2) phase is formed. Between θ = 0.5 and θ = 0.67 this phase coexists with and transforms into a (3 × 3) phase as indicated by a splitting of the (1212) beams in[11̄] direction until at θ = 0.67 the c(2 × 2) phase has completely converted into the (3 × 3) phase. The fractional order beam intensities as well as their angular profiles were recorded as a function of temperature at fixed coverages; they clearly show continuous order-disorder transitions for both hydrogen phases. The corresponding phase diagrams were constructed from the points of inflection of the intensity-temperature curves as well as from the onset of the broadening of the angular beam profiles. Critical temperatures of 245 (±5) K and 265 (±5) K were derived for the c(2 × 2) and the (3 × 3) phases, respectively. The results are discussed and qualitatively interpreted in terms of the interaction energies between the adsorbed hydrogen atoms." @default.
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- W2087195685 date "1982-05-01" @default.
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- W2087195685 title "Phase transitions of a two-dimensional chemisorbed system: H on Fe(110)" @default.
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- W2087195685 doi "https://doi.org/10.1016/0039-6028(82)90506-4" @default.
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