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• W2087256231 abstract "In this work, the oxygen-doped C3N4@TiO2 (O-C3N4@TiO2) composites with quasi-shell-core nanostructure were fabricated by coating a monolayer or multilayers of O-C3N4 onto the surface of TiO2 nanoparticles. Compared with the C3N4@TiO2 quasi-shell-core nanocomposite, the O-C3N4@TiO2 quasi-shell-core nanocomposite exhibits a significant promotion of the photoelectrochemical and photocatalytic performance of TiO2, owing to the interfacial chemical bonds formed between the hydroxyl residues on TiO2 surface and the oxidizing groups on O-C3N4 surface induced by oxygen doping. The experimental results of UV/Vis diffuse reflectance spectroscopy, electrochemical impedance spectroscopy, photoluminescence spectroscopy and excited state electron attenuation spectroscopy further reveal that this interfacial chemical bonds formed between O-C3N4 and TiO2 can become effective transfer channels for the photogenerated electrons, help to capture the electrons from the valence band of O-C3N4 and rapidly quench the photogenerated holes of TiO2, thereby effectively reducing the recombination efficiency of the photogenerated electrons and holes." @default.
• W2087256231 created "2016-06-24" @default.
• W2087256231 creator A5064095491 @default.
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• W2087256231 date "2014-10-01" @default.
• W2087256231 modified "2023-09-28" @default.
• W2087256231 title "Effect of oxygen-doped C3N4 on the separation capability of the photoinduced electron-hole pairs generated by O-C3N4@TiO2 with quasi-shell-core nanostructure" @default.
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• W2087256231 doi "https://doi.org/10.1016/j.electacta.2014.08.095" @default.
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