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• W2087291294 abstract "Abstract The oxidation of isobutene has been investigated for the first time in a jet-stirred reactor at high temperature (∼800-l230K) and at l,5and 10 atm. Molecular species concentration profiles of O2, H2, CO, CO2, CH2O, CH4, C2H2, C2H4, C2H6, C3H4 (allene and propyne), C3H6, acetone, acrolein, methacrolein, I-C4H8, i-C4H8, 1,3-C4H6, l-butyne, isoprene, 2-methyl-l-butene, 2-methyl-2-butene, and benzene were obtained by probe sampling and GC analysis. The oxidation of isobutene in these conditions and the ignition of isobutene-oxygen-argon mixtures in a shock-tube were modeled using a detailed kinetic reaction mechanism (l 10 species and 743 reactions, most of them reversible). The proposed mechanism, also validated for the oxidation of CH4, C2H2, C2H4, C2H4, C3H6, acetaldehyde, ethylene oxide, and natural gas blends in the same conditions, is able to predict experimental results obtained in our high-pressure jet stirred reactor and the ignition delays measured behind a reflected shock wave. Two routes to benzene formation have been delineated: (a) the addition of propargyl radicals to allene, and (b) the recombination of propargyl radicals. Sensitivity analyses and reaction path analyses are used to interpret the present results." @default.
• W2087291294 created "2016-06-24" @default.
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• W2087291294 date "1998-08-01" @default.
• W2087291294 modified "2023-10-17" @default.
• W2087291294 title "Isobutene Oxidation and Ignition: Experimental and Detailed Kinetic Modeling Study" @default.
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• W2087291294 doi "https://doi.org/10.1080/00102209808952053" @default.
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