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• W2087321123 abstract "A plate-type catalytic membrane reactor (PCMR) was prepared for the water-gas shift (WGS) reaction. The nickel metal catalyst with a disk-shape was placed on a disk-type membrane without a metal cage or mesh to hold the catalyst in the reactor. The WGS reaction in a PCMR was experimentally investigated using a simulated feed from coal gasification as a function of feed pressure (up to 1.1 MPa) and GHSV (up to 20 000 h− 1). The stronger adsorption of CO on the Pd membrane seems to be responsible for the greater reduction in the hydrogen permeating flux, which was a more power inhibitor than steam. When S/C = 2.0 and GHSV = 5000 h− 1, 81% of the hydrogen had permeated through the membrane at del-P = 1.0 MPa and 400 °C and the CO conversion increased by 26%, when compared with no hydrogen separation (del-P = 0.0 MPa). The CO conversion decreased by 8.1% when GHSV was increased from 5000 h− 1 to 17 000 h− 1." @default.
• W2087321123 created "2016-06-24" @default.
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• W2087321123 date "2013-02-01" @default.
• W2087321123 modified "2023-10-17" @default.
• W2087321123 title "Water-gas shift reaction in a plate-type Pd-membrane reactor over a nickel metal catalyst" @default.
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• W2087321123 doi "https://doi.org/10.1016/j.fuproc.2012.07.013" @default.
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