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• W2087360680 abstract "H atoms, O atoms, and OH radicals were identified in the catalytic decomposition of H2∕O2 mixtures on heated polycrystalline tungsten surfaces. In order to suppress the oxidization of the tungsten catalyzer surfaces, the H2∕O2 pressure ratio was kept more than 83, while the catalyzer temperature was kept below 2000K. The absolute density of H atoms was determined by a vacuum-ultraviolet laser absorption technique, while one-photon and two-photon laser-induced fluorescence techniques were employed to extend the dynamic range. Since the O-atom density was much smaller, only a vacuum-ultraviolet laser-induced fluorescence technique could be used for the detection. The absolute density could be estimated by comparing the induced fluorescence intensity with that for H atoms. OH radicals could be identified by a laser-induced fluorescence technique in the ultraviolet region. The absolute density was determined by comparing the induced fluorescence intensity with that of Rayleigh scattering caused by Ar. The H-atom density decreased with the increase in the O2 partial pressure stepwisely. The O-atom density increased with the O2 partial pressure monotonously, but the increase was rather slow at low O2 pressures. The OH-radical density showed saturation against the O2 partial pressure. These results can be explained by the change in the coverage conditions of the catalyzer surfaces." @default.
• W2087360680 created "2016-06-24" @default.
• W2087360680 creator A5034827268 @default.
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• W2087360680 date "2008-02-01" @default.
• W2087360680 modified "2023-10-12" @default.
• W2087360680 title "Production and detection of reducing and oxidizing radicals in the catalytic decomposition of H2∕O2 mixtures on heated tungsten surfaces" @default.
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• W2087360680 doi "https://doi.org/10.1063/1.2841510" @default.
• W2087360680 hasPublicationYear "2008" @default.
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