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• W2087525987 abstract "The chromium(III) nitrito complex trans-Cr(cyclam)(ONO)(2)(+) (1) is a very promising photochemical precursor for nitric oxide delivery to physiological targets. Here, we demonstrate that visible wavelength excitation of 1 in solutions containing thiol reductants such as the biological antioxidant glutathione (GSH) leads to permanent reaction even under anaerobic conditions, resulting in high quantum yield NO release. The nitric oxide formed under such conditions is sufficient, even at muM concentrations of 1 and using a low-intensity light source, to activate the enzyme soluble guanylyl cyclase (sGC). We also demonstrate that photolysis of 1 in the nM concentration range with a portable blue LED leads to vasorelaxation of porcine coronary arterial rings, a process also attributed to the NO activation of sGC." @default.
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• W2087525987 date "2009-12-01" @default.
• W2087525987 modified "2023-10-16" @default.
• W2087525987 title "Nitric Oxide Photogeneration from <i>trans</i>-Cr(cyclam)(ONO)₂⁺ in a Reducing Environment. Activation of Soluble Guanylyl Cyclase and Arterial Vasorelaxation" @default.
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• W2087525987 doi "https://doi.org/10.1021/jm9013357" @default.
• W2087525987 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19950902" @default.
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