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• W2088049092 abstract "A Jahn–Teller linear-plus-quadratic Hamiltonian is shown to account for most of the observed band positions and intensities in the absorption and emission spectra of Ag3. Coupling parameters obtained for a simultaneous fit to absorption and emission results are k=1.93, g=0.25 for the E′ ground state and k=0.19, g=0.02 for the E″ excited state. At higher vibrational energies, simple Jahn–Teller calculations predict fewer bands than observed. Calculations including spin–orbit coupling with larger linear coupling partially quenched by the Ham effect offer a reasonable explanation for this higher energy structure. Splittings and intensity sharing at lower vibrational energies, however, demand higher-order Jahn–Teller coupling, indicating the need for more extensive calculation simultaneously incorporating quadratic Jahn–Teller effects, spin–orbit coupling, and perhaps anharmonicity." @default.
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• W2088049092 date "1994-05-01" @default.
• W2088049092 modified "2023-10-16" @default.
• W2088049092 title "On the assignment of Jahn–Teller effects in the ultraviolet absorption spectrum of Ag3" @default.
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• W2088049092 doi "https://doi.org/10.1063/1.467093" @default.
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