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- W2088595812 abstract "The theory of the electronic matrix elements of the orbit–lattice interaction is developed with a view to its application to the case of high-spin ferrous iron. Spin–lattice transitions are classified according to their electronic matrix elements, and the necessary selection rules are determined. The ideas developed are used to discuss Fe2 + in octahedral, tetragonally distorted octahedral, and square-planar environments. It is concluded that partial quenching of the orbit–lattice interaction will occur in a square-planar environment. The line broadening observed in the Mössbauer spectrum of gillespite (BaFeSi4O10), in which iron is square planar coordinated by oxygens, is attributed to this effect. Spin–orbit coupling coefficients for the terms arising from 5D in a ligand field of D4 symmetry are tabulated." @default.
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- W2088595812 date "1968-04-01" @default.
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- W2088595812 title "Electronic Factors in the Paramagnetic Relaxation of High‐Spin Fe2 +" @default.
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- W2088595812 doi "https://doi.org/10.1063/1.1669598" @default.
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