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• W2088687962 abstract "Being a best known thermoelectric material and a topological insulator at ambient condition, magic bismuth telluride (${mathrm{Bi}}_{2}{mathrm{Te}}_{3}$) under pressure transforms into several superconducting phases, whose structures remain unsolved for decades. Here, we have solved the two long-puzzling low high-pressure phases as seven- and eightfold monoclinic structures, respectively, through particle-swarm optimization technique on crystal structure prediction. Above 14.4 GPa, we experimentally discovered that ${mathrm{Bi}}_{2}{mathrm{Te}}_{3}$ unexpectedly develops into a Bi-Te substitutional alloy by adopting a body-centered cubic disordered structure stable at least up to 52.1 GPa. The continuously monoclinic distortion leads to the ultimate formation of the Bi-Te alloy, which is attributed to the $mathrm{Bi}ensuremath{rightarrow}mathrm{Te}$ charge transfer under pressure. Our research provides a route to find alloys made of nonmetallic elements for a variety of applications." @default.
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• W2088687962 date "2011-04-08" @default.
• W2088687962 modified "2023-09-30" @default.
• W2088687962 title "Substitutional Alloy of Bi and Te at High Pressure" @default.
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• W2088687962 doi "https://doi.org/10.1103/physrevlett.106.145501" @default.
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