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- W2088890092 abstract "In a recent paper, Mungan et al. [Phys. Rev. B 54, 9204 (1996)] have proposed a model of ``universal two-state reorientational dynamics of diatomic hydrides in fcc salt crystals,'' based experimentally on an observed disappearance of librational ir absorption around 150 K. For the only presented example of ${mathrm{OH}}^{mathrm{ensuremath{-}}}$ defects in RbCl hosts, we show by comparison to our measurements that this claimed disappearance is not valid even up to $T=350$ K. Moreover, we show by accurate spectral data of two other examples $({mathrm{OH}}^{mathrm{ensuremath{-}}}$ and ${mathrm{OD}}^{mathrm{ensuremath{-}}}$ in KBr) that the claimed universal validity of the proposed ``thermally activated jump-rotational-diffusion model'' is not true for ${mathrm{OH}}^{mathrm{ensuremath{-}}}$ and ${mathrm{OD}}^{mathrm{ensuremath{-}}}$ in fcc alkali-chloride and bromide crystals and that there is no contrast to the ${mathrm{OH}}^{mathrm{ensuremath{-}}}/{mathrm{OD}}^{mathrm{ensuremath{-}}}$ dynamic behavior in bcc CsCl hosts." @default.
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- W2088890092 date "1997-09-01" @default.
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- W2088890092 title "Comment on “Universal two-state reorientational dynamics of diatomic hydrides in fcc salt crystals”" @default.
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- W2088890092 doi "https://doi.org/10.1103/physrevb.56.6345" @default.
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