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- W2089169255 abstract "Abstract CF 3 SO 3 H‐catalyzed reaction of 5‐alkyl‐( R )‐substituted diphenylhomobenzoquinone epoxides (R = Me, i Pr, t Bu) provided indenoquinones, a cyclopenta[ b ]chromene‐2‐carbaldehyde, and furan‐3(2 H )‐ones through novel cationic domino rearrangements depending on the R substituents. The mechanisms of these reactions were described by a combination of various key steps involving (i) transannular cyclization of the endo ‐phenyl group, (ii) epoxide and cyclopropane ring opening, (iii) ring contraction of the original quinone frame, (iv) dehydration and intramolecular S E 2/S N 2‐Ar cyclization, as well as (v) possible pseudopericyclic cheletropic decarbonylation." @default.
- W2089169255 created "2016-06-24" @default.
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- W2089169255 date "2012-06-14" @default.
- W2089169255 modified "2023-10-10" @default.
- W2089169255 title "Versatile Domino Rearrangement of Diphenylhomobenzoquinone Epoxides Induced by CF3SO3H" @default.
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- W2089169255 doi "https://doi.org/10.1002/ejoc.201200455" @default.
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