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• W2089455364 abstract "Stilbene radical anions (St•-) in the second excited doublet state generated by a pulse radiolysis−laser flash photolysis combined method undergo unimolecular isomerization from c-St•- to t-St•-, photoelectron ejection, and electron transfer to biphenyl added as a quencher. From the selective electron transfer from the St•- D2 states to biphenyl (Bp), kBpτ = 10.7 and 17.8 M-1 were obtained where kBp and τ denote the rate constants of the electron transfer and the lifetimes of the c-St•- and t-St•- D2 states, respectively. The τ values are estimated to be approximately 1.5 ± 0.4 ns and 2.5 ± 0.7 ns for the c-St•- and t-St•- D2 states, respectively, from kBpτ assuming the diffusion-controlled rate constant for kBp. The shorter τ of the c-St•- D2 state is attributed to isomerization via twisting about the central CC double bond. The τ values of the c-St•- and t-St•- D2 states are 1 order of magnitude longer than those of c-St•+ and t-St•+ D2 states. The transient phenomena of the D2 states of c-St•- and t-St•- are discussed in terms of their lifetimes, structures, energies, and reaction processes." @default.
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• W2089455364 date "1996-01-01" @default.
• W2089455364 modified "2023-10-14" @default.
• W2089455364 title "Stilbene Radical Anions in the Excited Doublet State" @default.
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• W2089455364 doi "https://doi.org/10.1021/jp960282i" @default.
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