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- W2089589034 abstract "Two-photon laser-induced fluorescence measurements of transition frequencies and lifetimes of laser-excited Na atoms are presented as a function of distance (2–3 nm) to metal surfaces of different roughness. We characterized the surface roughness by fitting a Gaussian height–height correlation function to force microscopic data. An unusually small red shift of the Na transition frequency of a few hundred megahertz was observed. In the framework of a quantum-mechanical linear optical response formalism we fitted the lifetime and the frequency shift data simultaneously to obtain effective parameters of a selvedge dielectric function. In that way we are able to take into account both surface roughness and nonlocality, which in turn result in the observed small frequency shifts." @default.
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- W2089589034 date "1997-08-15" @default.
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- W2089589034 title "Frequency shifts and lifetime changes of sodium atoms near rough metal surfaces" @default.
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- W2089589034 doi "https://doi.org/10.1364/ol.22.001262" @default.
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