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• W2089681412 abstract "Highly cross-linked polystyrene microgel colloids dispersed in an index and density matching solvent provide a system with hard-sphere-like interactions, where gravity effects are effectively minimized. They are a suitable target for time-resolved observations of solidification in purely repulsive systems. We have investigated the crystallization kinetics at increasing undercooling using time resolved light scattering. Crystallization starts always with the formation of compressed, structurally heterogeneous precursor domains. In the coexistence region the precursors, after being converted into true crystallites, start growing fast by assimilating particles from the melt. The resulting polycrystalline material consists of high quality crystals and seems not to undergo long time-scale rearrangements. As the particle concentration grows, the higher undercooling and reduced particle mobility increasingly compromise the conversion-growth process. The growth of crystallites relies then on much slower ripeninglike processes, while refining of the crystal structure is detected up to the longest observed times." @default.
• W2089681412 created "2016-06-24" @default.
• W2089681412 creator A5039734988 @default.
• W2089681412 creator A5039978758 @default.
• W2089681412 creator A5049963264 @default.
• W2089681412 date "2009-02-27" @default.
• W2089681412 modified "2023-10-02" @default.
• W2089681412 title "Crystallization kinetics of polydisperse hard-sphere-like microgel colloids: Ripening dominated crystal growth above melting" @default.
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• W2089681412 doi "https://doi.org/10.1063/1.3078310" @default.
• W2089681412 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19256610" @default.
• W2089681412 hasPublicationYear "2009" @default.
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