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- W2089891431 abstract "The time separation of experimental surface energy on Pt–Rh bimetallic catalysts, together with the time-independent rate constants for adsorption and desorption of O2, CO, and CO2 on them, is described, applying the reversed-flow version of inverse gas chromatography. The standard free energy of adsorption ΔG⦵ and its probability density function over time, together with the geometrical mean of the London parts of the total surface free energy (γL1γL2)1/2 of the adsorbed probe and the solid surface, accompanied by the relevant probability density functions over time are also calculated. The time-resolved phenomena lead to quite varying values of ΔG⦵, (γL1γL2)1/2, and the distribution functions as time passes, their maximum values being given by the catalyst containing a Pt:Rh = 3:1 weight ratio of the active phase for all adsorbed gases. The conclusion is reached that the surface energy measured as described can be used as a good measure for catalyst characterization." @default.
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- W2089891431 date "2004-02-01" @default.
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- W2089891431 title "Surface energy of solid catalysts measured by inverse gas chromatography" @default.
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- W2089891431 doi "https://doi.org/10.1016/j.jcis.2003.07.037" @default.
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