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- W2089986018 abstract "Noble metal nanoparticles (NPs) are spontaneously enfolded by aqueous coordination networks generated by reacting 2,5-dimercapto-1,3,4-thiadiazole (DMcT) with silver nanostructures in zero-oxidation state, and finally form novel hollow Au@Ag@infinite coordination polymers core–shell nanostructures (Au@Ag@void@ICPs). In this synthesis, DMcT molecules not only act as the bridging ligands but also directly oxidize Ag0 to Ag+ ions for the formation of amorphous DMcT–Ag ICPs. And, the sizes of the shell and void of Au@Ag@void@ICPs can be facilely tuned by modulating the amount of DMcT and the size ratio of Au@Ag NPs, respectively. Due to the high structural tailorability of DMcT–Ag ICPs, multi-encapsulation of Au@Ag NPs with either small organic molecules or biological macromolecules (e.g., enzymes) can be achieved to fabricate multi-functional core–shell nanostructures. A case in point is that a highly sensitive biosensor of H2O2 with a wider detection window has been constructed based on the prepared metal NPs–ICPs–enzyme composites and resonance Raman scattering. This study provides not only a new template for tailoring hollow core–shell nanomaterials but also a versatile platform for chemical (bio) sensing." @default.
- W2089986018 created "2016-06-24" @default.
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- W2089986018 date "2014-07-30" @default.
- W2089986018 modified "2023-10-17" @default.
- W2089986018 title "Inclusion of guest materials in aqueous coordination network shells spontaneously generated by reacting 2,5-dimercapto-1,3,4-thiadiazole with nanoscale metallic silver" @default.
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- W2089986018 doi "https://doi.org/10.1039/c4ra07281b" @default.
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