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- W2090136013 abstract "The radiative decays of vibrationally excited DCO+ ions produced by dissociative ionization of CD3CDO have been investigated using the monitor ion technique in a Fourier transform ion cyclotron resonance spectrometer. The radiative lifetimes of the ν1 (v = 1, 2) and ν3 (v = 1) stretching modes have been determined. For the CO stretching ν3 the experimental lifetime (24 ± 2.5 ms) is in good agreement with the theoretical values calculated for DCO+ and HCO+. For the CD stretching ν1 the experimental lifetimes (112 ± 22 ms) for v = 2 and (226 ± 45 ms) for v = 1 are about four times larger than the theoretical values. The disagreement between experiment and theory is possibly due to a strong coupling of ν1 with a long lived state which has not been taken into account in the calculations. For the bending mode ν2, only a lower limit of the very long lifetime could be evaluated." @default.
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- W2090136013 date "1999-04-01" @default.
- W2090136013 modified "2023-09-24" @default.
- W2090136013 title "Radiative lifetime measurements of the CO and CD stretching modes in DCO" @default.
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- W2090136013 doi "https://doi.org/10.1016/s1387-3806(98)14113-1" @default.
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