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- W2090358400 abstract "The roles played by the conformational disordering of alkyl chains in determining the aggregation states of matter are reviewed for liquid crystalline materials from a thermodynamic perspective. Entropy, which is one of the most macroscopic concepts but which has a clear microscopic meaning, provides crucial microscopic information for complex systems for which a microscopic description is hard to establish. Starting from structural implication by absolute (third-law) entropy for crystalline solids, the existence of successive phase transitions caused by the successive conformational melting of alkyl chains in discotic mesogens is explained. An experimental basis is given for the quasi-binary picture of thermotropic liquid crystals, i.e., the highly disordered alkyl chains behave like a second component (solvent). A novel entropy transfer between the components of a molecule and the resulting alkyl chains as entropy reservoir mechanism are explained for cubic mesogens." @default.
- W2090358400 created "2016-06-24" @default.
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- W2090358400 date "2003-01-01" @default.
- W2090358400 modified "2023-10-15" @default.
- W2090358400 title "Alkyl chains acting as entropy reservoir in liquid crystalline materials" @default.
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- W2090358400 doi "https://doi.org/10.1002/tcr.10046" @default.
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