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• W2090523941 abstract "The theoretical development for one-dimensional, coupled migration of solutes with different ionic mobilities through clay soils that behave as ion-restrictive membranes, referred to as clay membrane barriers (CMBs), is presented. The transport formulation is based on principles of irreversible thermodynamics and accounts explicitly for coupling effects of hyperfiltration (ultrafiltration) and chemico-osmotic counter-advection associated with clay membrane behavior in the absence of electrical current. Since, by definition, no solute can enter a perfect or ideal membrane, the concept of an implicit coupling effect, such that the effective salt-diffusion coefficient, Ds* approaches zero as the chemico-osmotic efficiency coefficient, omega approaches unity is introduced. The theoretical development also illustrates that, even in the absence of membrane behavior, traditional advective-dispersive transport theory based on a constant value of Ds* for the solutes may not be appropriate for simulating transient transport in reactive (ion exchanging) systems. This potential limitation is illustrated through simulations for solute mass flux involving the migration of a binary salt solution (KCl) through a clay barrier with exchange sites saturated with a single exchangeable cation (e.g., Na+) that enters the pore solution upon ion exchange with the salt cation (K+)." @default.
• W2090523941 created "2016-06-24" @default.
• W2090523941 creator A5019621111 @default.
• W2090523941 creator A5032089344 @default.
• W2090523941 date "2002-12-01" @default.
• W2090523941 modified "2023-09-25" @default.
• W2090523941 title "Theory for reactive solute transport through clay membrane barriers" @default.
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• W2090523941 doi "https://doi.org/10.1016/s0169-7722(02)00041-4" @default.
• W2090523941 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/12487418" @default.
• W2090523941 hasPublicationYear "2002" @default.
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