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- W2090572406 abstract "The catalytic effects of MoCl3–LiCl–KCl and NiCl2–LiCl–KCl molten salts were studied for the hydroliquefaction of Morwell brown and Taiheiyo subbituminous coals at 400 °C for 1 h in a batch reactor with an initial hydrogen pressure of 9.8 MPa. The conversion to pyridine-soluble materials and the yield of hexane-soluble materials (HS) with the MoCl3 catalyst were 82 and 42% for Morwell coal, and 84 and 61% for Taiheiyo coal, respectively. The conversion and HS yield with the NiCl2 catalyst were 87 and 43% for Morwell coal, and 82 and 56% for Taiheiyo coal, respectively. The HS yield of the catalytic runs was about 2.6–3.2 times higher than that of noncatalytic runs. This finding established the effectiveness of the two new catalysts for the hydroliquefaction of brown and subbituminous coals. Detailed analyses of the reaction products have revealed that these catalysts promoted a depolymerization of the coals and strongly catalyzed the hydrocracking of polynuclear aromatic structures of heavy products into hydroaromatic and aromatic structures with smaller ring sizes. Most of these smaller hydroaromatic and aromatic structures did not undergo much further ring-opening reactions. This accounts for the high HS selectivity of the catalysts." @default.
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- W2090572406 date "1986-11-01" @default.
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- W2090572406 title "Catalytic Effects of MoCl<sub>3</sub>- and NiCl<sub>2</sub>-Containing Molten Salts for Hydroliquefaction of Morwell Brown and Taiheiyo Subbituminous Coals" @default.
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- W2090572406 doi "https://doi.org/10.1246/bcsj.59.3643" @default.
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