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• W2090680103 abstract "We present high-frequency high-field electron paramagnetic resonance (EPR) measurements on the dodecanuclear manganese complex Mn12-bromoacetate (Mn12-BrAc). The crystal-field parameters are found to be identical to those of the original compound Mn12-acetate (Mn12-Ac). A detailed analysis of the frequency and temperature dependence of anomalous peaks observed in the EPR spectra of Mn12-BrAc enables us to locate the S=9 manifold at about 40 K above the Ms= +/-10 ground state of this nominally S=10 system. This is very close to the Ms = +/-6 state of the S = 10 manifold, thus suggesting pathways for the thermally assisted magnetization dynamics and related properties. Finally, the EPR fine structures recently attributed to disorder associated with the acetic acid of crystallization in Mn12-Ac are absent in the present measurements, thus suggesting that the Mn12-BrAc complex represents a more suitable candidate for measurements of quantum effects in high symmetry S=10 SMMs." @default.
• W2090680103 created "2016-06-24" @default.
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• W2090680103 date "2004-08-31" @default.
• W2090680103 modified "2023-09-26" @default.
• W2090680103 title "Evidence for the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mi>S</mml:mi><mml:mo>=</mml:mo><mml:mn>9</mml:mn></mml:mrow></mml:math>excited state in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mi mathvariant=normal>Mn</mml:mi><mml:mn>12</mml:mn></mml:msub></mml:math>-bromoacetate measured by electron paramagnetic resonance" @default.
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• W2090680103 doi "https://doi.org/10.1103/physrevb.70.054426" @default.
• W2090680103 hasPublicationYear "2004" @default.
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