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- W2090762286 abstract "Abstract An unprecedented reactivity has been introduced to 3‐isopropyl‐1,4‐benzodiazepine‐2,5‐dione thanks to N ‐Boc activation. Under basic conditions, a transannular rearrangement occurred by ring contraction to furnish a 3‐aminoquinoline‐2,4‐dione with good to excellent enantiomeric purity. Depending on the nature of the base, either enantiomer can be obtained in a stereocontrolled manner. This enantiodivergent synthesis could be assigned to the conformational equilibrium of the starting material, which was studied with the help of DFT calculations." @default.
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- W2090762286 date "2011-02-21" @default.
- W2090762286 modified "2023-10-14" @default.
- W2090762286 title "Enantiodivergent Transannular Rearrangement of 3-Isopropyl-1,4-benzodiazepine-2,5-dione by Memory of Chirality" @default.
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- W2090762286 doi "https://doi.org/10.1002/ejoc.201100030" @default.
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