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- W2090906592 abstract "F-type centres can be produced by contacting the MgO surface with Mg vapour at ≈ 873 K. CO adsorption at 77 K on such a MgMgO system was studied by infrared spectroscopy. Comparison with CO adsorption at 77 K on undoped MgO shows that, besides the monomeric, dimeric and trimeric species observed on pure MgO, new carbonylic entities are formed on Mg doped MgO. Two isomeric structures of C2O22−, acetylenediolate ions and other carbonylic compounds which have Mgm(CO)n and/or possibly CO− formula are produced. C2O22− species are very sensitive to oxygen. These data confirm that F-type centres produced on MgMgO are very reactive toward simple molecules and strengthen the opinion that the spectroscopic and adsorptive properties of such special sites cannot be confused with those of active centres present on the surface of thermally activated MgO." @default.
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- W2090906592 date "1991-09-01" @default.
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- W2090906592 title "Novel dimeric species produced by CO interaction with surface F-type centres on Mg-doped MgO: an IR study" @default.
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- W2090906592 doi "https://doi.org/10.1016/0254-0584(91)90038-v" @default.
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