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• W2090952004 abstract "Abstract The energetics of La‐doping in BaTiO 3 are reported for both (electronic) donor‐doping with the creation of Ti 3+ cations and ionic doping with the creation of Ti vacancies. The experiments (for samples prepared in air) and simulations demonstrate that ionic doping is the preferred mechanism for all concentrations of La‐doping. The apparent disagreement with electrical conduction of these ionic doped samples is explained by subsequent oxygen‐loss, which leads to the creation of Ti 3+ cations. Simulations show that oxygen‐loss is much more favorable in the ionic‐doped system than undoped BaTiO 3 due to the unique local structure created around the defect site. These findings resolve the so‐called “donor‐doping” anomaly in BaTiO 3 and explain the source of semiconductivity in positive temperature coefficient of resistance (PTCR) BaTiO 3 thermistors." @default.
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• W2090952004 date "2013-03-06" @default.
• W2090952004 modified "2023-10-18" @default.
• W2090952004 title "Energetics of Donor-Doping, Metal Vacancies, and Oxygen-Loss in A-Site Rare-Earth-Doped BaTiO₃" @default.
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• W2090952004 doi "https://doi.org/10.1002/adfm.201203147" @default.
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